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1.
J Environ Radioact ; 274: 107399, 2024 Apr.
Article in English | MEDLINE | ID: mdl-38442434

ABSTRACT

The article considers the issues of working out the suitable approaches for identifying zones with the presence of underground near-surface waters with increased concentrations of tritium discharged into a surface reservoir. The following methods were used as possible methods: determination of tritium content in snow cover, determination of tritium content in vegetation in the form of tritium of free water and organically bound tritium, determination of tritium content in river water and coastal vegetation. The studies were carried out at a previously identified site where groundwater with a tritium concentration of up to 6000 Bq/l is present, located in the vicinity of the city of Obninsk (Kaluga region, Russia). As a result of the conducted research, it was concluded that the analysis of the distribution of tritium in vegetation is an excellent methodological technique for identifying areas of location of near-surface underground waters contaminated with tritium. As a control parameter, both the concentration of tritium in the free water of plants and the content of organically bound tritium can be used. To detect underground tritium contamination the most promising use is the following indicator - the content of OBT in the shoots of woody plants. This parameter is very informative, and the sampling procedure for its determination has no seasonal restrictions, unlike such parameters as the content of tritium in grass and leaves, the content of tritium in snow cover, surface waters, which are preferably collected only in summer or winter. It should be noted that the control of surface waters of the groundwater discharge zone may not be a sufficiently informative indicator for identifying areas of polluted water inflow, since it depends on the ratio of the volumes of leaking polluted groundwater and the annual flow of the watercourse.


Subject(s)
Radiation Monitoring , Tritium/analysis , Radiation Monitoring/methods , Ecosystem , Wood/chemistry , Water
2.
J Environ Radioact ; 247: 106865, 2022 Jun.
Article in English | MEDLINE | ID: mdl-35316687

ABSTRACT

This study is devoted to the estimation of radionuclides global fallout levels in the soils of Commonwealth of Independent States (CIS) and Eastern Europe territory as a result of nuclear explosions. 58 standard soil samples were used, which were selected in different soil and climatic areas of the territory of CIS and Eastern Europe in 1978-2018. All samples were measured by gamma spectrometry. Determination of plutonium isotopes and strontium was performed according to the method of the joint determination of these radionuclides from one sample. IN the samples considered in this work, the content of 60Co, 154Eu, 155Eu was below the detection limits, which were 0.4; 1.0 and 1.0, respectively. Natural radionuclides analysis results indicated that the obtained samples are typical soil samples without its abnormal contents. The content of 137Cs, 90Sr, 239+240Pu in a 20 cm soil layer due to global fallout is (3.9 ± 1.7), (2.2 ± 0.8), (0.18 ± 0.08) Bq/kg respectively, which considering the distribution of these radionuclides by depth and average soil density is (1.2 ± 0.5) kBq/m2 for 137Cs, (0.42 ± 0.15) kBq/m2- 90Sr and (55.0 ± 24.0) Bq/m2- 239+240Pu. The isotopic ratios137Cs/90Sr and 137Cs/239+240Pu for the territory of CIS and Eastern Europe are at the level (2.0 ± 0.71) and (25 ± 15), respectively.


Subject(s)
Plutonium , Radiation Monitoring , Soil Pollutants, Radioactive , Europe, Eastern , Plutonium/analysis , Radiation Monitoring/methods , Soil , Soil Pollutants, Radioactive/analysis
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